Correlating Superconducting Qubit Performance Losses to Sidewall Near-Field Scattering via Terahertz Nanophotonics

  1. Richard H. J. Kim,
  2. Samuel J. Haeuser,
  3. Joong-Mok Park,
  4. Randall K. Chan,
  5. Jin-Su Oh,
  6. Thomas Koschny,
  7. Lin Zhou,
  8. Matthew J. Kramer,
  9. Akshay A. Murthy,
  10. Mustafa Bal,
  11. Francesco Crisa,
  12. Sabrina Garattoni,
  13. Shaojiang Zhu,
  14. Andrei Lunin,
  15. David Olaya,
  16. Peter Hopkins,
  17. Alex Romanenko,
  18. Anna Grassellino,
  19. and Jigang Wang
Elucidating dielectric losses, structural heterogeneity, and interface imperfections is critical for improving coherence in superconducting qubits. However, most diagnostics rely on
destructive electron microscopy or low-throughput millikelvin quantum measurements. Here, we demonstrate noninvasive terahertz (THz) nano-imaging/-spectroscopy of encapsulated niobium transmon qubits, revealing sidewall near-field scattering that correlates with qubit coherence. We further employ a THz hyperspectral line scan to probe dielectric responses and field participation at Al junction interfaces. These findings highlight the promise of THz near-field methods as a high-throughput proxy characterization tool for guiding material selection and optimizing processing protocols to improve qubit and quantum circuit performance.

Floquet-Engineered Fast SNAP gates in weakly coupled cQED systems

  1. Xinyuan You,
  2. Andy C. Y. Li,
  3. Tanay Roy,
  4. Shaojiang Zhu,
  5. Alexander Romanenko,
  6. Anna Grassellino,
  7. Yao Lu,
  8. and Srivatsan Chakram
Superconducting cavities with high quality factors, coupled to a fixed-frequency transmon, provide a state-of-the-art platform for quantum information storage and manipulation. The
commonly used selective number-dependent arbitrary phase (SNAP) gate faces significant challenges in ultra-high-coherence cavities, where the weak dispersive shifts necessary for preserving high coherence typically result in prolonged gate times. Here, we propose a protocol to achieve high-fidelity SNAP gates that are orders of magnitude faster than the standard implementation, surpassing the speed limit set by the bare dispersive shift. We achieve this enhancement by dynamically amplifying the dispersive coupling via sideband interactions, followed by quantum optimal control on the Floquet-engineered system. We also present a unified perturbation theory that explains both the gate acceleration and the associated benign drive-induced decoherence, corroborated by Floquet-Markov simulations. These results pave the way for the experimental realization of high-fidelity, selective control of weakly coupled, high-coherence cavities, and expanding the scope of optimal control techniques to a broader class of Floquet quantum systems.

Ultracoherent superconducting cavity-based multiqudit platform with error-resilient control

  1. Taeyoon Kim,
  2. Tanay Roy,
  3. Xinyuan You,
  4. Andy C. Y. Li,
  5. Henry Lamm,
  6. Oleg Pronitchev,
  7. Mustafa Bal,
  8. Sabrina Garattoni,
  9. Francesco Crisa,
  10. Daniel Bafia,
  11. Doga Kurkcuoglu,
  12. Roman Pilipenko,
  13. Paul Heidler,
  14. Nicholas Bornman,
  15. David van Zanten,
  16. Silvia Zorzetti,
  17. Roni Harnik,
  18. Akshay Murthy,
  19. Shaojiang Zhu,
  20. Changqing Wang,
  21. Andre Vallieres,
  22. Ziwen Huang,
  23. Jens Koch,
  24. Anna Grassellino,
  25. Srivatsan Chakram,
  26. Alexander Romanenko,
  27. and Yao Lu
Superconducting radio-frequency (SRF) cavities offer a promising platform for quantum computing due to their long coherence times and large accessible Hilbert spaces, yet integrating
nonlinear elements like transmons for control often introduces additional loss. We report a multimode quantum system based on a 2-cell elliptical shaped SRF cavity, comprising two cavity modes weakly coupled to an ancillary transmon circuit, designed to preserve coherence while enabling efficient control of the cavity modes. We mitigate the detrimental effects of the transmon decoherence through careful design optimization that reduces transmon-cavity couplings and participation in the dielectric substrate and lossy interfaces, to achieve single-photon lifetimes of 20.6 ms and 15.6 ms for the two modes, and a pure dephasing time exceeding 40 ms. This marks an order-of-magnitude improvement over prior 3D multimode memories. Leveraging sideband interactions and novel error-resilient protocols, including measurement-based correction and post-selection, we achieve high-fidelity control over quantum states. This enables the preparation of Fock states up to N=20 with fidelities exceeding 95%, the highest reported to date to the authors‘ knowledge, as well as two-mode entanglement with coherence-limited fidelities reaching up to 99.9% after post-selection. These results establish our platform as a robust foundation for quantum information processing, allowing for future extensions to high-dimensional qudit encodings.

Demonstrating magnetic field robustness and reducing temporal T1 noise in transmon qubits through magnetic field engineering

  1. Bektur Abdisatarov,
  2. Tanay Roy,
  3. Daniel Bafia,
  4. Roman Pilipenko,
  5. Matthew Julian Dubiel,
  6. David van Zanten,
  7. Shaojiang Zhu,
  8. Mustafa Bal,
  9. Grigory Eremeev,
  10. Hani Elsayed-Ali,
  11. Akshay Murty,
  12. Alexander Romanenko,
  13. and Anna Grassellino
The coherence of superconducting transmon qubits is often disrupted by fluctuations in the energy relaxation time (T1), limiting their performance for quantum computing. While background
magnetic fields can be harmful to superconducting devices, we demonstrate that both trapped magnetic flux and externally applied static magnetic fields can suppress temporal fluctuations in T1 without significantly degrading its average value or qubit frequency. Using a three-axis Helmholtz coil system, we applied calibrated magnetic fields perpendicular to the qubit plane during cooldown and operation. Remarkably, transmon qubits based on tantalum-capped niobium (Nb/Ta) capacitive pads and aluminum-based Josephson junctions (JJs) maintained T1 lifetimes near 300 {\mu}s even when cooled in fields as high as 600 mG. Both trapped flux up to 600 mG and applied fields up to 400 mG reduced T1 fluctuations by more than a factor of two, while higher field strengths caused rapid coherence degradation. We attribute this stabilization to the polarization of paramagnetic impurities, the role of trapped flux as a sink for non-equilibrium quasiparticles (QPs), and partial saturation of fluctuating two-level systems (TLSs). These findings challenge the conventional view that magnetic fields are inherently detrimental and introduce a strategy for mitigating noise in superconducting qubits, offering a practical path toward more stable and scalable quantum systems.

Identifying Materials-Level Sources of Performance Variation in Superconducting Transmon Qubits

  1. Akshay A. Murthy,
  2. Mustafa Bal,
  3. Michael J. Bedzyk,
  4. Hilal Cansizoglu,
  5. Randall K. Chan,
  6. Venkat Chandrasekhar,
  7. Francesco Crisa,
  8. Amlan Datta,
  9. Yanpei Deng,
  10. Celeo D. Matute Diaz,
  11. Vinayak P. Dravid,
  12. David A. Garcia-Wetten,
  13. Sabrina Garattoni,
  14. Sunil Ghimire,
  15. Dominic P. Goronzy,
  16. Sebastian de Graaf,
  17. Sam Haeuser,
  18. Mark C. Hersam,
  19. Dieter Isheim,
  20. Kamal Joshi,
  21. Richard Kim,
  22. Saagar Kolachina,
  23. Cameron J. Kopas,
  24. Matthew J. Kramer,
  25. Ella O. Lachman,
  26. Jaeyel Lee,
  27. Peter G. Lim,
  28. Andrei Lunin,
  29. William Mah,
  30. Jayss Marshall,
  31. Josh Y. Mutus,
  32. Jin-Su Oh,
  33. David Olaya,
  34. David P. Pappas,
  35. Joong-mok Park,
  36. Ruslan Prozorov,
  37. Roberto dos Reis,
  38. David N. Seidman,
  39. Zuhawn Sung,
  40. Makariy Tanatar,
  41. Mitchell J. Walker,
  42. Jigang Wang,
  43. Haotian Wu,
  44. Lin Zhou,
  45. Shaojiang Zhu,
  46. Anna Grassellino,
  47. and Alexander Romanenko
The Superconducting Materials and Systems (SQMS) Center, a DOE National Quantum Information Science Research Center, has conducted a comprehensive and coordinated study using superconducting
transmon qubit chips with known performance metrics to identify the underlying materials-level sources of device-to-device performance variation. Following qubit coherence measurements, these qubits of varying base superconducting metals and substrates have been examined with various nondestructive and invasive material characterization techniques at Northwestern University, Ames National Laboratory, and Fermilab as part of a blind study. We find trends in variations of the depth of the etched substrate trench, the thickness of the surface oxide, and the geometry of the sidewall, which when combined, lead to correlations with the T1 lifetime across different devices. In addition, we provide a list of features that varied from device to device, for which the impact on performance requires further studies. Finally, we identify two low-temperature characterization techniques that may potentially serve as proxy tools for qubit measurements. These insights provide materials-oriented solutions to not only reduce performance variations across neighboring devices, but also to engineer and fabricate devices with optimal geometries to achieve performance metrics beyond the state-of-the-art values.

Disentangling the Impact of Quasiparticles and Two-Level Systems on the Statistics of Superconducting Qubit Lifetime

  1. Shaojiang Zhu,
  2. Xinyuan You,
  3. Ugur Alyanak,
  4. Mustafa Bal,
  5. Francesco Crisa,
  6. Sabrina Garattoni,
  7. Andrei Lunin,
  8. Roman Pilipenko,
  9. Akshay Murthy,
  10. Alexander Romanenko,
  11. and Anna Grassellino
Temporal fluctuations in the superconducting qubit lifetime, T1, bring up additional challenges in building a fault-tolerant quantum computer. While the exact mechanisms remain unclear,
T1 fluctuations are generally attributed to the strong coupling between the qubit and a few near-resonant two-level systems (TLSs) that can exchange energy with an assemble of thermally fluctuating two-level fluctuators (TLFs) at low frequencies. Here, we report T1 measurements on the qubits with different geometrical footprints and surface dielectrics as a function of the temperature. By analyzing the noise spectrum of the qubit depolarization rate, Γ1=1/T1, we can disentangle the impact of TLSs, non-equilibrium quasiparticles (QPs), and equilibrium (thermally excited) QPs on the variance in Γ1. We find that Γ1 variances in the qubit with a small footprint are more susceptible to the QP and TLS fluctuations than those in the large-footprint qubits. Furthermore, the QP-induced variances in all qubits are consistent with the theoretical framework of QP diffusion and fluctuation. We suggest these findings can offer valuable insights for future qubit design and engineering optimization.

Evaluating radiation impact on transmon qubits in above and underground facilities

  1. Francesco De Dominicis,
  2. Tanay Roy,
  3. Ambra Mariani,
  4. Mustafa Bal,
  5. Nicola Casali,
  6. Ivan Colantoni,
  7. Francesco Crisa,
  8. Angelo Cruciani,
  9. Fernando Ferroni,
  10. Dounia L Helis,
  11. Lorenzo Pagnanini,
  12. Valerio Pettinacci,
  13. Roman M Pilipenko,
  14. Stefano Pirro,
  15. Andrei Puiu,
  16. Alexander Romanenko,
  17. David v Zanten,
  18. Shaojiang Zhu,
  19. Anna Grassellino,
  20. and Laura Cardani
Superconducting qubits can be sensitive to abrupt energy deposits caused by cosmic rays and ambient radioactivity. Previous studies have focused on understanding possible correlated
effects over time and distance due to cosmic rays. In this study, for the first time, we directly compare the response of a transmon qubit measured initially at the Fermilab SQMS above-ground facilities and then at the deep underground Gran Sasso Laboratory (INFN-LNGS, Italy). We observe same average qubit lifetime T1 of roughly 80 microseconds at above and underground facilities. We then apply a fast decay detection protocol and investigate the time structure, sensitivity and relative rates of triggered events due to radiation versus intrinsic noise, comparing above and underground performance of several high-coherence qubits. Using gamma sources of variable activity we calibrate the response of the qubit to different levels of radiation in an environment with minimal background radiation. Results indicate that qubits respond to a strong gamma source and it is possible to detect particle impacts. However, when comparing above and underground results, we do not observe a difference in radiation induced-like events for these sapphire and niobium-based transmon qubits. We conclude that the majority of these events are not radiation related and to be attributed to other noise sources which by far dominate single qubit errors in modern transmon qubits.

Fast ZZ-Free Entangling Gates for Superconducting Qubits Assisted by a Driven Resonator

  1. Ziwen Huang,
  2. Taeyoon Kim,
  3. Tanay Roy,
  4. Yao Lu,
  5. Alexander Romanenko,
  6. Shaojiang Zhu,
  7. and Anna Grassellino
Engineering high-fidelity two-qubit gates is an indispensable step toward practical quantum computing. For superconducting quantum platforms, one important setback is the stray interaction
between qubits, which causes significant coherent errors. For transmon qubits, protocols for mitigating such errors usually involve fine-tuning the hardware parameters or introducing usually noisy flux-tunable couplers. In this work, we propose a simple scheme to cancel these stray interactions. The coupler used for such cancellation is a driven high-coherence resonator, where the amplitude and frequency of the drive serve as control knobs. Through the resonator-induced-phase (RIP) interaction, the static ZZ coupling can be entirely neutralized. We numerically show that such a scheme can enable short and high-fidelity entangling gates, including cross-resonance CNOT gates within 40 ns and adiabatic CZ gates within 140 ns. Our architecture is not only ZZ free but also contains no extra noisy components, such that it preserves the coherence times of fixed-frequency transmon qubits. With the state-of-the-art coherence times, the error of our cross-resonance CNOT gate can be reduced to below 1e-4.

Systematic Improvements in Transmon Qubit Coherence Enabled by Niobium Surface Encapsulation

  1. Mustafa Bal,
  2. Akshay A. Murthy,
  3. Shaojiang Zhu,
  4. Francesco Crisa,
  5. Xinyuan You,
  6. Ziwen Huang,
  7. Tanay Roy,
  8. Jaeyel Lee,
  9. David van Zanten,
  10. Roman Pilipenko,
  11. Ivan Nekrashevich,
  12. Daniel Bafia,
  13. Yulia Krasnikova,
  14. Cameron J. Kopas,
  15. Ella O. Lachman,
  16. Duncan Miller,
  17. Josh Y. Mutus,
  18. Matthew J. Reagor,
  19. Hilal Cansizoglu,
  20. Jayss Marshall,
  21. David P. Pappas,
  22. Kim Vu,
  23. Kameshwar Yadavalli,
  24. Jin-Su Oh,
  25. Lin Zhou,
  26. Matthew J. Kramer,
  27. Dominic P. Goronzy,
  28. Carlos G. Torres-Castanedo,
  29. Graham Pritchard,
  30. Vinayak P. Dravid,
  31. James M. Rondinelli,
  32. Michael J. Bedzyk,
  33. Mark C. Hersam,
  34. John Zasadzinski,
  35. Jens Koch,
  36. James A. Sauls,
  37. Alexander Romanenko,
  38. and Anna Grassellino
We present a novel transmon qubit fabrication technique that yields systematic improvements in T1 coherence times. We fabricate devices using an encapsulation strategy that involves
passivating the surface of niobium and thereby preventing the formation of its lossy surface oxide. By maintaining the same superconducting metal and only varying the surface structure, this comparative investigation examining different capping materials and film substrates across different qubit foundries definitively demonstrates the detrimental impact that niobium oxides have on the coherence times of superconducting qubits, compared to native oxides of tantalum, aluminum or titanium nitride. Our surface-encapsulated niobium qubit devices exhibit T1 coherence times 2 to 5 times longer than baseline niobium qubit devices with native niobium oxides. When capping niobium with tantalum, we obtain median qubit lifetimes above 200 microseconds. Our comparative structural and chemical analysis suggests that amorphous niobium suboxides may induce higher losses. These results are in line with high-accuracy measurements of the niobium oxide loss tangent obtained with ultra-high Q superconducting radiofrequency (SRF) cavities. This new surface encapsulation strategy enables further reduction of dielectric losses via passivation with ambient-stable materials, while preserving fabrication and scalable manufacturability thanks to the compatibility with silicon processes.

Stabilizing and improving qubit coherence by engineering noise spectrum of two-level systems

  1. Xinyuan You,
  2. Ziwen Huang,
  3. Ugur Alyanak,
  4. Alexander Romanenko,
  5. Anna Grassellino,
  6. and Shaojiang Zhu
The coherence times of many widely used superconducting qubits are limited by material defects that can be modeled as an ensemble of two-level systems (TLSs). Among them, charge fluctuators
inside amorphous oxide layers are believed to contribute to both low-frequency 1/f charge noise and high-frequency dielectric loss, causing fast qubit dephasing and relaxation. Here, we propose to mitigate those noise channels by engineering the relevant TLS noise spectral densities. Specifically, our protocols smooth the high-frequency noise spectrum and suppress the low-frequency noise amplitude via relaxing and dephasing the TLSs, respectively. As a result, we predict a drastic stabilization in qubit lifetime and an increase in qubit pure dephasing time. Our detailed analysis of feasible experimental implementations shows that the improvement is not compromised by spurious coupling from the applied noise to the qubit.