Transmon qubits are a cornerstone of modern superconducting quantum computing platforms. Temporal fluctuations of energy relaxation in these qubits are widely attributed to microscopictwo-level systems (TLSs) in device dielectrics and interfaces, yet isolating individual defects typically relies on tuning the qubit or the TLS into resonance. We demonstrate a novel spectroscopy method for fixed-frequency transmons based on multilevel relaxation: repeated preparation of the second excited state and simultaneous T1 extraction of the first and second excited states reveals characteristic correlations in the decay rates of adjacent transitions. From these correlations we identify one or more dominant TLSs and reconstruct their frequency drift over time. Remarkably, we find that TLSs detuned by ≳100MHz from the qubit transition can still significantly influence relaxation. The proposed method provides a powerful tool for TLS spectroscopy without the need to tune the transmon frequency, either via a flux-tunable inductor or AC-Stark shifts.
Niobium metal occupies nearly 100% of the volume of a typical 2D transmon device. While the aluminum Josephson junction is of utmost importance, maintaining quantum coherence acrossthe entire device means that pair-breaking in Nb leads, capacitive pads, and readout resonators can be a major source of decoherence. The established contributors are surface oxides and hydroxides, as well as absorbed hydrogen and oxygen. Metal encapsulation of freshly grown surfaces with non-oxidizing metals, preferably without breaking the vacuum, is a successful strategy to mitigate these issues. While the positive effects of encapsulation are undeniable, it is important to understand its impact on the macroscopic behavior of niobium films. We present a comprehensive study of the bulk superconducting properties of Nb thin films encapsulated with gold and palladium/gold, and compare them to those of bare Nb films. Magneto-optical imaging, magnetization, resistivity, and London and Campbell penetration depth measurements reveal significant differences in encapsulated samples. Both sputtered, and epitaxial Au-capped films exhibit the highest residual resistivity ratio and superconducting transition temperature, as well as the lowest upper critical field, London penetration depth, and critical current. These results are in good agreement with the microscopic theory of anisotropic normal and superconducting states of Nb. We conclude that pair-breaking in the bulk of niobium films, driven by disorder throughout the film rather than just at the surface, is a significant source of quantum decoherence in transmons. We also conclude that gold capping not only passivates the surface but also affects the properties of the entire film, significantly reducing the scattering rate due to defects likely induced by surface diffusion if the film is not protected immediately after fabrication.
Ionizing radiation has emerged as a potential limiting factor for superconducting quantum processors, inducing quasiparticle bursts and correlated errors that challenge fault-tolerantoperation. Atmospheric muons are particularly problematic due to their high energy and penetration power, making passive shielding ineffective. Therefore, monitoring the real-time muon flux is crucial to guide the development of alternative error-correction or protection strategies. We present the design, simulation, and first operation of a cryogenic muon-tagging system based on Kinetic Inductance Detectors (KIDs) for integration with superconducting quantum processors. The system consists of two KIDs arranged in a vertical stack and operated at ~20 mK. Monte Carlo simulations based on Geant4 guided the prototype design and provided reference expectations for muon-tagging efficiency and accidental coincidences due to ambient γ-rays. We measured a muon-induced coincidence rate among the top and bottom detectors of (192 ± 9) × 10−3 events/s, in excellent agreement with the Monte Carlo prediction. The prototype achieves a muon-tagging efficiency of about 90% with negligible dead time. These results demonstrate the feasibility of operating a muon-tagging system at millikelvin temperatures and open the path toward its integration with multi-qubit chips to veto or correct muon-induced errors in real time.
Elucidating dielectric losses, structural heterogeneity, and interface imperfections is critical for improving coherence in superconducting qubits. However, most diagnostics rely ondestructive electron microscopy or low-throughput millikelvin quantum measurements. Here, we demonstrate noninvasive terahertz (THz) nano-imaging/-spectroscopy of encapsulated niobium transmon qubits, revealing sidewall near-field scattering that correlates with qubit coherence. We further employ a THz hyperspectral line scan to probe dielectric responses and field participation at Al junction interfaces. These findings highlight the promise of THz near-field methods as a high-throughput proxy characterization tool for guiding material selection and optimizing processing protocols to improve qubit and quantum circuit performance.
Superconducting radio-frequency (SRF) cavities offer a promising platform for quantum computing due to their long coherence times and large accessible Hilbert spaces, yet integratingnonlinear elements like transmons for control often introduces additional loss. We report a multimode quantum system based on a 2-cell elliptical shaped SRF cavity, comprising two cavity modes weakly coupled to an ancillary transmon circuit, designed to preserve coherence while enabling efficient control of the cavity modes. We mitigate the detrimental effects of the transmon decoherence through careful design optimization that reduces transmon-cavity couplings and participation in the dielectric substrate and lossy interfaces, to achieve single-photon lifetimes of 20.6 ms and 15.6 ms for the two modes, and a pure dephasing time exceeding 40 ms. This marks an order-of-magnitude improvement over prior 3D multimode memories. Leveraging sideband interactions and novel error-resilient protocols, including measurement-based correction and post-selection, we achieve high-fidelity control over quantum states. This enables the preparation of Fock states up to N=20 with fidelities exceeding 95%, the highest reported to date to the authors‘ knowledge, as well as two-mode entanglement with coherence-limited fidelities reaching up to 99.9% after post-selection. These results establish our platform as a robust foundation for quantum information processing, allowing for future extensions to high-dimensional qudit encodings.
The Superconducting Materials and Systems (SQMS) Center, a DOE National Quantum Information Science Research Center, has conducted a comprehensive and coordinated study using superconductingtransmon qubit chips with known performance metrics to identify the underlying materials-level sources of device-to-device performance variation. Following qubit coherence measurements, these qubits of varying base superconducting metals and substrates have been examined with various nondestructive and invasive material characterization techniques at Northwestern University, Ames National Laboratory, and Fermilab as part of a blind study. We find trends in variations of the depth of the etched substrate trench, the thickness of the surface oxide, and the geometry of the sidewall, which when combined, lead to correlations with the T1 lifetime across different devices. In addition, we provide a list of features that varied from device to device, for which the impact on performance requires further studies. Finally, we identify two low-temperature characterization techniques that may potentially serve as proxy tools for qubit measurements. These insights provide materials-oriented solutions to not only reduce performance variations across neighboring devices, but also to engineer and fabricate devices with optimal geometries to achieve performance metrics beyond the state-of-the-art values.
Temporal fluctuations in the superconducting qubit lifetime, T1, bring up additional challenges in building a fault-tolerant quantum computer. While the exact mechanisms remain unclear,T1 fluctuations are generally attributed to the strong coupling between the qubit and a few near-resonant two-level systems (TLSs) that can exchange energy with an assemble of thermally fluctuating two-level fluctuators (TLFs) at low frequencies. Here, we report T1 measurements on the qubits with different geometrical footprints and surface dielectrics as a function of the temperature. By analyzing the noise spectrum of the qubit depolarization rate, Γ1=1/T1, we can disentangle the impact of TLSs, non-equilibrium quasiparticles (QPs), and equilibrium (thermally excited) QPs on the variance in Γ1. We find that Γ1 variances in the qubit with a small footprint are more susceptible to the QP and TLS fluctuations than those in the large-footprint qubits. Furthermore, the QP-induced variances in all qubits are consistent with the theoretical framework of QP diffusion and fluctuation. We suggest these findings can offer valuable insights for future qubit design and engineering optimization.