Identifying Materials-Level Sources of Performance Variation in Superconducting Transmon Qubits

  1. Akshay A. Murthy,
  2. Mustafa Bal,
  3. Michael J. Bedzyk,
  4. Hilal Cansizoglu,
  5. Randall K. Chan,
  6. Venkat Chandrasekhar,
  7. Francesco Crisa,
  8. Amlan Datta,
  9. Yanpei Deng,
  10. Celeo D. Matute Diaz,
  11. Vinayak P. Dravid,
  12. David A. Garcia-Wetten,
  13. Sabrina Garattoni,
  14. Sunil Ghimire,
  15. Dominic P. Goronzy,
  16. Sebastian de Graaf,
  17. Sam Haeuser,
  18. Mark C. Hersam,
  19. Dieter Isheim,
  20. Kamal Joshi,
  21. Richard Kim,
  22. Saagar Kolachina,
  23. Cameron J. Kopas,
  24. Matthew J. Kramer,
  25. Ella O. Lachman,
  26. Jaeyel Lee,
  27. Peter G. Lim,
  28. Andrei Lunin,
  29. William Mah,
  30. Jayss Marshall,
  31. Josh Y. Mutus,
  32. Jin-Su Oh,
  33. David Olaya,
  34. David P. Pappas,
  35. Joong-mok Park,
  36. Ruslan Prozorov,
  37. Roberto dos Reis,
  38. David N. Seidman,
  39. Zuhawn Sung,
  40. Makariy Tanatar,
  41. Mitchell J. Walker,
  42. Jigang Wang,
  43. Haotian Wu,
  44. Lin Zhou,
  45. Shaojiang Zhu,
  46. Anna Grassellino,
  47. and Alexander Romanenko
The Superconducting Materials and Systems (SQMS) Center, a DOE National Quantum Information Science Research Center, has conducted a comprehensive and coordinated study using superconducting
transmon qubit chips with known performance metrics to identify the underlying materials-level sources of device-to-device performance variation. Following qubit coherence measurements, these qubits of varying base superconducting metals and substrates have been examined with various nondestructive and invasive material characterization techniques at Northwestern University, Ames National Laboratory, and Fermilab as part of a blind study. We find trends in variations of the depth of the etched substrate trench, the thickness of the surface oxide, and the geometry of the sidewall, which when combined, lead to correlations with the T1 lifetime across different devices. In addition, we provide a list of features that varied from device to device, for which the impact on performance requires further studies. Finally, we identify two low-temperature characterization techniques that may potentially serve as proxy tools for qubit measurements. These insights provide materials-oriented solutions to not only reduce performance variations across neighboring devices, but also to engineer and fabricate devices with optimal geometries to achieve performance metrics beyond the state-of-the-art values.

Quasiparticle spectroscopy, transport, and magnetic properties of Nb films used in superconducting transmon qubits

  1. Kamal R. Joshi,
  2. Sunil Ghimire,
  3. Makariy A. Tanatar,
  4. Amlan Datta,
  5. Jin-Su Oh,
  6. Lin Zhou,
  7. Cameron J. Kopas,
  8. Jayss Marshall,
  9. Josh Y. Mutus,
  10. Julie Slaughter,
  11. Matthew J. Kramer,
  12. James A. Sauls,
  13. and Ruslan Prozorov
Niobium thin films on silicon substrate used in the fabrication of superconducting qubits have been characterized using scanning and transmission electron microscopy, electrical transport,
magnetization, quasiparticle spectroscopy, and real-space real-time magneto-optical imaging. We study niobium films to provide an example of a comprehensive analytical set that may benefit superconducting circuits such as those used in quantum computers. The films show outstanding superconducting transition temperature of Tc=9.35 K and a fairly clean superconducting gap, along with superfluid density enhanced at intermediate temperatures. These observations are consistent with the recent theory of anisotropic strong-coupling superconductivity in Nb. However, the response to the magnetic field is complicated, exhibiting significantly irreversible behavior and insufficient heat conductance leading to thermo-magnetic instabilities. These may present an issue for further improvement of transmon quantum coherence. Possible mitigation strategies are discussed.