Precision measurement of the microwave dielectric loss of sapphire in the quantum regime with parts-per-billion sensitivity

  1. Alexander P. Read,
  2. Benjamin J. Chapman,
  3. Chan U Lei,
  4. Jacob C. Curtis,
  5. Suhas Ganjam,
  6. Lev Krayzman,
  7. Luigi Frunzio,
  8. and Robert J. Schoelkopf
Dielectric loss is known to limit state-of-the-art superconducting qubit lifetimes. Recent experiments imply upper bounds on bulk dielectric loss tangents on the order of 100 parts-per-billion,
but because these inferences are drawn from fully fabricated devices with many loss channels, they do not definitively implicate or exonerate the dielectric. To resolve this ambiguity, we have devised a measurement method capable of separating and resolving bulk dielectric loss with a sensitivity at the level of 5 parts-per-billion. The method, which we call the dielectric dipper, involves the in-situ insertion of a dielectric sample into a high-quality microwave cavity mode. Smoothly varying the sample’s participation in the cavity mode enables a differential measurement of the sample’s dielectric loss tangent. The dielectric dipper can probe the low-power behavior of dielectrics at cryogenic temperatures, and does so without the need for any lithographic process, enabling controlled comparisons of substrate materials and processing techniques. We demonstrate the method with measurements of EFG sapphire, from which we infer a bulk loss tangent of 62(7)×10−9 and a substrate-air interface loss tangent of 12(2)×10−4. For a typical transmon, this bulk loss tangent would limit device quality factors to less than 20 million, suggesting that bulk loss is likely the dominant loss mechanism in the longest-lived transmons on sapphire. We also demonstrate this method on HEMEX sapphire and bound its bulk loss tangent to be less than 15(5)×10−9. As this bound is about four times smaller than the bulk loss tangent of EFG sapphire, use of HEMEX sapphire as a substrate would lift the bulk dielectric coherence limit of a typical transmon qubit to several milliseconds.

Observation of wave-packet branching through an engineered conical intersection

  1. Christopher S. Wang,
  2. Nicholas E. Frattini,
  3. Benjamin J. Chapman,
  4. Shruti Puri,
  5. Steven M. Girvin,
  6. Michel H. Devoret,
  7. and Robert J. Schoelkopf
In chemical reactions, the interplay between coherent evolution and dissipation is central to determining key properties such as the rate and yield. Of particular interest are cases
where two potential energy surfaces cross at features known as conical intersections (CIs), resulting in nonadiabatic dynamics that may promote ultrafast and highly efficient reactions when rovibrational damping is present. A prominent chemical reaction that involves a CI is the cis-trans isomerization reaction in rhodopsin, which is crucial to vision. CIs in real molecular systems are typically investigated via optical pump-probe spectroscopy, which has demanding spectral bandwidth and temporal resolution requirements, and where precise control of the environment is challenging. A complementary approach for understanding chemical reactions is to use quantum simulators that can provide access to a wider range of observables, though thus far combining strongly interacting linear (rovibrational) and nonlinear (electronic) degrees of freedom with engineered dissipation has yet to be demonstrated. Here, we create a tunable CI in a hybrid qubit-oscillator circuit QED processor and simultaneously track both a reactive wave-packet and electronic qubit in the time-domain. We identify dephasing of the electronic qubit as the mechanism that drives wave-packet branching along the reactive coordinate in our model. Furthermore, we directly observe enhanced branching when the wave-packet passes through the CI. Thus, the forces that influence a chemical reaction can be viewed as an effective measurement induced dephasing rate that depends on the position of the wave-packet relative to the CI. Our results set the groundwork for more complex simulations of chemical dynamics, offering deeper insight into the role of dissipation in determining macroscopic quantities of interest such as the quantum yield of a chemical reaction.

Fast Universal Control of an Oscillator with Weak Dispersive Coupling to a Qubit

  1. Alec Eickbusch,
  2. Volodymyr Sivak,
  3. Andy Z. Ding,
  4. Salvatore S. Elder,
  5. Shantanu R. Jha,
  6. Jayameenakshi Venkatraman,
  7. Baptiste Royer,
  8. S. M. Girvin,
  9. Robert J. Schoelkopf,
  10. and Michel H. Devoret
Efficient quantum control of an oscillator is necessary for many bosonic applications including error-corrected computation, quantum-enhanced sensing, robust quantum communication,
and quantum simulation. For these applications, oscillator control is often realized through off-resonant hybridization to a qubit with dispersive shift χ where typical operation times of 2π/χ are routinely assumed. Here, we challenge this assumption by introducing and demonstrating a novel control method with typical operation times over an order of magnitude faster than 2π/χ. Using large auxiliary displacements of the oscillator to enhance gate speed, we introduce a universal gate set with built-in dynamical decoupling consisting of fast conditional displacements and qubit rotations. We demonstrate the method using a superconducting cavity weakly coupled to a transmon qubit in a regime where previously known methods would fail. Our demonstrations include preparation of a single-photon state 30 times faster than 2π/χ with 98±1(%) fidelity and preparation of squeezed vacuum with a squeezing level of 11.1 dB, the largest intracavity squeezing reported in the microwave regime. Finally, we demonstrate fast measurement-free preparation of logical states for the binomial and Gottesman-Kitaev-Preskill (GKP) code, and we identify possible fidelity limiting mechanisms including oscillator dephasing.

Quantum control of bosonic modes with superconducting circuits

  1. Wen-Long Ma,
  2. Shruti Puri,
  3. Robert J. Schoelkopf,
  4. Michel H. Devoret,
  5. S. M. Girvin,
  6. and Liang Jiang
Bosonic modes have wide applications in various quantum technologies, such as optical photons for quantum communication, magnons in spin ensembles for quantum information storage and
mechanical modes for reversible microwave-to-optical quantum transduction. There is emerging interest in utilizing bosonic modes for quantum information processing, with circuit quantum electrodynamics (circuit QED) as one of the leading architectures. Quantum information can be encoded into subspaces of a bosonic superconducting cavity mode with long coherence time. However, standard Gaussian operations (e.g., beam splitting and two-mode squeezing) are insufficient for universal quantum computing. The major challenge is to introduce additional nonlinear control beyond Gaussian operations without adding significant bosonic loss or decoherence. Here we review recent advances in universal control of a single bosonic code with superconducting circuits, including unitary control, quantum feedback control, driven-dissipative control and holonomic dissipative control. Entangling different bosonic modes with various approaches is also discussed.

Single-shot number-resolved detection of microwave photons with error mitigation

  1. Jacob C. Curtis,
  2. Connor T. Hann,
  3. Salvatore S. Elder,
  4. Christopher S. Wang,
  5. Luigi Frunzio,
  6. Liang Jiang,
  7. and Robert J. Schoelkopf
Single-photon detectors are ubiquitous and integral components of photonic quantum cryptography, communication, and computation. Many applications, however, require not only detecting
the presence of any photons, but distinguishing the number present with a single shot. Here, we implement a single-shot, high-fidelity photon number-resolving detector of up to 15 microwave photons in a cavity-qubit circuit QED platform. This detector functions by measuring a series of generalized parity operators which make up the bits in the binary decomposition of the photon number. Our protocol consists of successive, independent measurements of each bit by entangling the ancilla with the cavity, then reading out and resetting the ancilla. Photon loss and ancilla readout errors can flip one or more bits, causing nontrivial errors in the outcome, but these errors have a traceable form which can be captured in a simple hidden Markov model. Relying on the independence of each bit measurement, we mitigate biases in the measurement result, showing good agreement with the predictions of the model. The mitigation improves the average total variation distance error of Fock states from 13.5% to 1.3%. We also show that the mitigation is efficiently scalable to an M-mode system provided that the errors are independent and sufficiently small. Our work motivates the development of new algorithms that utilize single-shot, high-fidelity PNR detectors.

High coherence superconducting microwave cavities with indium bump bonding

  1. Chan U Lei,
  2. Lev Krayzman,
  3. Suhas Ganjam,
  4. Luigi Frunzio,
  5. and Robert J. Schoelkopf
Low-loss cavities are important in building high-coherence superconducting quantum computers. Generating high quality joints between parts is crucial to the realization of a scalable
quantum computer using the circuit quantum electrodynamics (cQED) framework. In this paper, we adapt the technique of indium bump bonding to the cQED architecture to realize high quality superconducting microwave joints between chips. We use this technique to fabricate compact superconducting cavities in the multilayer microwave integrated quantum circuits (MMIQC) architecture and achieve single photon quality factor over 300 million or single-photon lifetimes approaching 5 ms. To quantify the performance of the resulting seam, we fabricate microwave stripline resonators in multiple sections connected by different numbers of bonds, resulting in a wide range of seam admittances. The measured quality factors combined with the designed seam admittances allow us to bound the conductance of the seam at gseam≥2×1010/(Ωm). Such a conductance should enable construction of micromachined superconducting cavities with quality factor of at least a billion. These results demonstrate the capability to construct very high quality microwave structures within the MMIQC architecture.

Path-Independent Quantum Gates with Noisy Ancilla

  1. Wen-Long Ma,
  2. Mengzhen Zhang,
  3. Yat Wong,
  4. Kyungjoo Noh,
  5. Serge Rosenblum,
  6. Philip Reinhold,
  7. Robert J. Schoelkopf,
  8. and Liang Jiang
Ancilla systems are often indispensable to universal control of a nearly isolated quantum system. However, ancilla systems are typically more vulnerable to environmental noise, which
limits the performance of such ancilla-assisted quantum control. To address this challenge of ancilla-induced decoherence, we propose a general framework that integrates quantum control and quantum error correction, so that we can achieve robust quantum gates resilient to ancilla noise. We introduce the path independence criterion for fault-tolerant quantum gates against ancilla errors. As an example, a path-independent gate is provided for superconducting circuits with a hardware-efficient design.

Quantum simulation of molecular vibronic spectra on a superconducting bosonic processor

  1. Christopher S. Wang,
  2. Jacob C. Curtis,
  3. Brian J. Lester,
  4. Yaxing Zhang,
  5. Yvonne Y. Gao,
  6. Jessica Freeze,
  7. Victor S. Batista,
  8. Patrick H. Vaccaro,
  9. Isaac L. Chuang,
  10. Luigi Frunzio,
  11. Liang Jiang,
  12. S. M. Girvin,
  13. and Robert J. Schoelkopf
The efficient simulation of quantum systems is a primary motivating factor for developing controllable quantum machines. A controllable bosonic machine is naturally suited for simulating
systems with underlying bosonic structure, exploiting both quantum interference and an intrinsically large Hilbert space. Here, we experimentally realize a bosonic superconducting processor that combines arbitrary state preparation, a complete set of Gaussian operations, plus an essential non-Gaussian resource – a novel single-shot photon number resolving measurement scheme – all in one device. We utilize these controls to simulate the bosonic problem of molecular vibronic spectra, extracting the corresponding Franck-Condon factors for photoelectron processes in H2O, O3, NO2, and SO2. Our results demonstrate the versatile capabilities of the circuit QED platform, which can be extended to include non-Gaussian operations for simulating an even wider class of bosonic systems.

High-fidelity measurement of qubits encoded in multilevel superconducting circuits

  1. Salvatore S. Elder,
  2. Christopher S. Wang,
  3. Philip Reinhold,
  4. Connor T. Hann,
  5. Kevin S. Chou,
  6. Brian J. Lester,
  7. Serge Rosenblum,
  8. Luigi Frunzio,
  9. Liang Jiang,
  10. and Robert J. Schoelkopf
Qubit measurements are central to quantum information processing. In the field of superconducting qubits, standard readout techniques are not only limited by the signal-to-noise ratio,
but also by state relaxation during the measurement. In this work, we demonstrate that the limitation due to relaxation can be suppressed by using the many-level Hilbert space of superconducting circuits: in a multilevel encoding, the measurement is only corrupted when multiple errors occur. Employing this technique, we show that we can directly resolve transmon gate errors at the level of one part in 103. Extending this idea, we apply the same principles to the measurement of a logical qubit encoded in a bosonic mode and detected with a transmon ancilla, implementing a proposal by Hann et al. [Phys. Rev. A \textbf{98} 022305 (2018)]. Qubit state assignments are made based on a sequence of repeated readouts, further reducing the overall infidelity. This approach is quite general and several encodings are studied; the codewords are more distinguishable when the distance between them is increased with respect to photon loss. The tradeoff between multiple readouts and state relaxation is explored and shown to be consistent with the photon-loss model. We report a logical assignment infidelity of 5.8×10−5 for a Fock-based encoding and 4.2×10−3 for a QEC code (the S=2,N=1 binomial code). Our results will not only improve the fidelity of quantum information applications, but also enable more precise characterization of process or gate errors.

Error-corrected gates on an encoded qubit

  1. Philip Reinhold,
  2. Serge Rosenblum,
  3. Wen-Long Ma,
  4. Luigi Frunzio,
  5. Liang Jiang,
  6. and Robert J. Schoelkopf
To solve classically hard problems, quantum computers need to be resilient to the influence of noise and decoherence. In such a fault-tolerant quantum computer, noise-induced errors
must be detected and corrected in real-time to prevent them from propagating between components. This requirement is especially pertinent while applying quantum gates, when the interaction between components can cause errors to quickly spread throughout the system. However, the large overhead involved in most fault-tolerant architectures makes implementing these systems a daunting task, which motivates the search for hardware-efficient alternatives. Here, we present a gate enacted by a multilevel ancilla transmon on a cavity-encoded logical qubit that is fault-tolerant with respect to decoherence in both the ancilla and the encoded qubit. We maintain the purity of the encoded qubit in the presence of ancilla errors by detecting those errors in real-time, and applying the appropriate corrections. We show a reduction of the logical gate error by a factor of two in the presence of naturally occurring decoherence, and demonstrate resilience against ancilla bit-flips and phase-flips by observing a sixfold suppression of the gate error with increased energy relaxation, and a fourfold suppression with increased dephasing noise. The results demonstrate that bosonic logical qubits can be controlled by error-prone ancilla qubits without inheriting the ancilla’s inferior performance. As such, error-corrected ancilla-enabled gates are an important step towards fully fault-tolerant processing of bosonic qubits.