Riccardo Comin

Encapsulation epitaxy of air-stable monolayer superconducting films for quantum circuits and qubits

  1. Xudong Zheng,
  2. Sameia Zaman,
  3. Kenan Zhang,
  4. Connor A Occhialini,
  5. Haowei Xu,
  6. Zhien Wang,
  7. Fangyuan Liu,
  8. Luiz Gustavo Pimenta Martins,
  9. Sejoon Lim,
  10. Tianyi Zhang,
  11. Tilo H. Yang,
  12. Jiangtao Wang,
  13. Yunyue Zhu,
  14. Zachariah Hennighausen,
  15. Sein Park,
  16. Steven Vitale,
  17. Kevin Tibbetts,
  18. Stephen Margiotta,
  19. Phillip Kim,
  20. Cong Su,
  21. Ju Li,
  22. Riccardo Comin,
  23. William D. Oliver,
  24. Joel I.J. Wang,
  25. and Jing Kong
Two-dimensional (2D) superconductors are an emerging platform for strongly correlated physics and quantum information science. Their reduced dimensionality, atomically flat interfaces,
and high crystallinity are attractive for realizing compact lumped-element devices in superconducting circuits. However, synthesizing large-area, monolayer 2D superconductors remains challenging because of their susceptibility to oxidation. Here, we report an „encapsulation epitaxy“ mechanism that enables the growth of large-area, air-stable, monolayer superconducting NbSe2 films and explore their use in superconducting quantum circuits. A 2D encapsulation layer, such as graphene or hexagonal boron nitride (hBN), pre-deposited on a 3D substrate (e.g., SiO2 or Si3N4), serves both as a template for epitaxial growth of monolayer NbSe2 (1L-NbSe2) underneath it and as a protective cover. This approach produces uniform, large-area (>1-inch) 1L-NbSe2 with greatly enhanced ambient stability, enabling device fabrication in air. The resulting 1L-graphene/NbSe2 heterostructures exhibit robust superconductivity (Tc ~ 1 K) and enhanced charge density wave order (TCDW ~ 177 K), indicative of high material quality. We further integrate 1L-NbSe2 into superconducting circuits using oxidation-free transfer and superconducting edge-contact techniques. The 1L-NbSe2 exhibits a measured kinetic inductance LK ~ 0.7 nH/square, making it suitable for quantum circuits requiring high-kinetic-inductance elements. Encapsulation epitaxy thus provides a route to air-stable 2D superconductors and van der Waals heterostructures, with potential for wafer-scale, monolithic fabrication of superconducting quantum circuitry.
arxiv pdf

Evolution of 1/f Flux Noise in Superconducting Qubits with Weak Magnetic Fields

  1. David A. Rower,
  2. Lamia Ateshian,
  3. Lauren H. Li,
  4. Max Hays,
  5. Dolev Bluvstein,
  6. Leon Ding,
  7. Bharath Kannan,
  8. Aziza Almanakly,
  9. Jochen Braumüller,
  10. David K. Kim,
  11. Alexander Melville,
  12. Bethany M. Niedzielski,
  13. Mollie E. Schwartz,
  14. Jonilyn L. Yoder,
  15. Terry P. Orlando,
  16. Joel I-Jan Wang,
  17. Simon Gustavsson,
  18. Jeffrey A. Grover,
  19. Kyle Serniak,
  20. Riccardo Comin,
  21. and William D. Oliver
The microscopic origin of 1/f magnetic flux noise in superconducting circuits has remained an open question for several decades despite extensive experimental and theoretical investigation.
Recent progress in superconducting devices for quantum information has highlighted the need to mitigate sources of qubit decoherence, driving a renewed interest in understanding the underlying noise mechanism(s). Though a consensus has emerged attributing flux noise to surface spins, their identity and interaction mechanisms remain unclear, prompting further study. Here we apply weak in-plane magnetic fields to a capacitively-shunted flux qubit (where the Zeeman splitting of surface spins lies below the device temperature) and study the flux-noise-limited qubit dephasing, revealing previously unexplored trends that may shed light on the dynamics behind the emergent 1/f noise. Notably, we observe an enhancement (suppression) of the spin-echo (Ramsey) pure dephasing time in fields up to B=100 G. With direct noise spectroscopy, we further observe a transition from a 1/f to approximately Lorentzian frequency dependence below 10 Hz and a reduction of the noise above 1 MHz with increasing magnetic field. We suggest that these trends are qualitatively consistent with an increase of spin cluster sizes with magnetic field. These results should help to inform a complete microscopic theory of 1/f flux noise in superconducting circuits.
arxiv pdf