Anomalous Frequency Shift in Low-Loss Superconducting Granular Aluminum Resonators

  1. Patrick Winkel,
  2. Daniil S. Antonenko,
  3. Vishakha Gupta,
  4. Neel Thakur,
  5. Pavel Kurilovich,
  6. Luigi Frunzio,
  7. Leonid I. Glazman,
  8. and Robert J. Schoelkopf
Superconducting high-kinetic inductance materials like granular aluminum (grAl) are a versatile part of the circuit quantum electrodynamics (cQED) toolbox, provided their losses at
microwave frequencies are low enough. To further advance the use of grAl in quantum devices, it is indispensable to identify the dominant loss mechanisms. The standard approach pairs electromagnetic simulations of resonator geometry with measured temperature and power dependence of resonance frequency and loss rate. Most materials follow the phenomenological theory of two-level systems (TLSs) at low temperatures, resulting in an initial decrease of the resonance frequency with increasing temperature. In our work, we observe an opposite behavior at the lowest temperatures: The resonance frequency initially increases with both temperature and readout power, contradicting the standard TLS model predictions. We are able to explain a part of the data by an alternative mechanism associated with the effect of superconducting quasiparticles in a granular system with spatially-nonuniform gap. Yet, the observed change in the resonance frequency with temperature is not matched by a proportional change in the loss rate. We also observe anomalous positive frequency responses following high-energy events, characterized by several time scales. While anomalous behavior has been reported previously in grAl, the disagreement with standard models is particularly visible in our devices thanks to their exceptionally low loss rates.

Low loss lumped-element inductors made from granular aluminum

  1. Vishakha Gupta,
  2. Patrick Winkel,
  3. Neel Thakur,
  4. Peter van Vlaanderen,
  5. Yanhao Wang,
  6. Suhas Ganjam,
  7. Luigi Frunzio,
  8. and Robert J. Schoelkopf
Lumped-element inductors are an integral component in the circuit QED toolbox. However, it is challenging to build inductors that are simultaneously compact, linear and low-loss with
standard approaches that either rely on the geometric inductance of superconducting thin films or on the kinetic inductance of Josephson junctions arrays. In this work, we overcome this challenge by utilizing the high kinetic inductance offered by superconducting granular aluminum (grAl). We demonstrate lumped-element inductors with a few nH of inductance that are up to 100 times more compact than inductors built from pure aluminum (Al). To characterize the properties of these linear inductors, we first report on the performance of lumped-element resonators built entirely out of grAl with sheet inductances varying from 30−320pH/sq and self-Kerr non-linearities of 0.2−20Hz/photon. Further, we demonstrate ex-situ integration of these grAl inductors into hybrid resonators with Al or tantalum (Ta) capacitor electrodes without increasing total internal losses. Interestingly, the measured internal quality factors systematically decrease with increasing room-temperature resistivity of the grAl film for all devices, indicating a trade-off between compactness and internal loss. For our lowest resistivity grAl films, we measure quality factors reaching 3.5×106 for the all-grAl devices and 4.5×106 for the hybrid grAl/Ta devices, similar to state-of-the-art quantum circuits. Our loss analysis suggests that the surface loss factor of grAl is similar to that of pure Al for our lowest resistivity films, while the increasing losses with resistivity could be explained by increasing conductor loss in the grAl film.