We experimentally study the transient dynamics of a dissipative superconducting qubit under periodic drive towards its nonequilibrium steady states. The corresponding stroboscopic evolution,given by the qubit states at times equal to integer multiples of the drive period, is determined by a (generically non-Hermitian) Floquet Liouvillian. The drive period controls both the transients across its non-Hermitian degeneracies and the resulting nonequilibrium steady states. These steady states can exhibit higher purity compared to those achieved with a constant drive. We further study the dependence of the steady states on the direction of parameter variation and relate these findings to the recent studies of dynamically encircling exceptional points. Our work provides a new approach to control non-Hermiticity in dissipative quantum systems and presents a new paradigm in quantum state preparation and stabilization.
Thermodynamics constrains changes to the energy of a system, both deliberate and random, via its first and second laws. When the system is not in equilibrium, fluctuation theorems suchas the Jarzynski equality further restrict the distributions of deliberate work done. Such fluctuation theorems have been experimentally verified in small, non-equilibrium quantum systems undergoing unitary or decohering dynamics. Yet, their validity in systems governed by a non-Hermitian Hamiltonian has long been contentious, due to the false premise of the Hamiltonian’s dual and equivalent roles in dynamics and energetics. Here we show that work fluctuations in a non-Hermitian qubit obey the Jarzynski equality even if its Hamiltonian has complex or purely imaginary eigenvalues. With post-selection on a dissipative superconducting circuit undergoing a cyclic parameter sweep, we experimentally quantify the work distribution using projective energy measurements and show that the fate of the Jarzynski equality is determined by the parity-time symmetry of, and the energetics that result from, the corresponding non-Hermitian, Floquet Hamiltonian. By distinguishing the energetics from non-Hermitian dynamics, our results provide the recipe for investigating the non-equilibrium quantum thermodynamics of such open systems.
Open quantum systems interacting with an environment exhibit dynamics described by the combination of dissipation and coherent Hamiltonian evolution. Taken together, these effects arecaptured by a Liouvillian superoperator. The degeneracies of the (generically non-Hermitian) Liouvillian are exceptional points, which are associated with critical dynamics as the system approaches steady state. We use a superconducting transmon circuit coupled to an engineered environment to observe two different types of Liouvillian exceptional points that arise either from the interplay of energy loss and decoherence or purely due to decoherence. By dynamically tuning the Liouvillian superoperators in real time we observe a non-Hermiticity-induced chiral state transfer. Our study motivates a new look at open quantum system dynamics from the vantage of Liouvillian exceptional points, enabling applications of non-Hermitian dynamics in the understanding and control of open quantum systems.