computational advantage over classical systems. A transformative opportunity on the horizon is merging the high-fidelity many-body evolution in analog simulators with the robust control and measurement of digital machines. Such a hybrid platform would unlock new capabilities in state preparation, characterization and dynamical control. Here, we embed digital quantum control in the analog evolution of a synthetic quantum material by entangling the lattice potential landscape of a Bose-Hubbard circuit with an ancilla qubit. This Hamiltonian-level control induces dynamics under a superposition of different lattice configurations and guides the many-body system to novel strongly-correlated states where different phases of matter coexist — ordering photons into superpositions of solid and fluid eigenstates. Leveraging hybrid control modalities, we adiabatically introduce disorder to localize the photons into an entangled cat state and enhance its coherence using a many-body echo technique. This work illustrates the potential for entangling quantum computers with quantum matter — synthetic and solid-state — for advantage in sensing and materials characterization.