Electron paramagnetic resonance (EPR) spectroscopy is an important technology in physics, chemistry, materials science, and biology. Sensitive detection with a small sample volume isa key objective in these areas, because it is crucial, for example, for the readout of a highly packed spin based quantum memory or the detection of unlabeled metalloproteins in a single cell. In conventional EPR spectrometers, the energy transfer from the spins to the cavity at a Purcell enhanced rate plays an essential role and requires the spins to be resonant with the cavity, however the size of the cavity (limited by the wavelength) makes it difficult to improve the spatial resolution. Here, we demonstrate a novel EPR spectrometer using a single artificial atom as a sensitive detector of spin magnetization. The artificial atom, a superconducting flux qubit, provides advantages both in terms of its quantum properties and its much stronger coupling with magnetic fields. We have achieved a sensitivity of ∼400 spins/Hz‾‾‾√ with a magnetic sensing volume around 10−14λ3 (50 femto-liters). This corresponds to an improvement of two-order of magnitude in the magnetic sensing volume compared with the best cavity based spectrometers while maintaining a similar sensitivity as those spectrometers . Our artificial atom is suitable for scaling down and thus paves the way for measuring single spins on the nanometer scale.
We report on spectra of circuit quantum electrodynamics (QED) systems in an intermediate regime that lies between the ultrastrong and deep strong coupling regimes, which have been reportedpreviously in the literature. Our experimental results, along with numerical simulations, demonstrate that as the coupling strength increases, the spectrum of a circuit-QED system undergoes multiple qualitative transformations, such that several ranges are identified, each with its own unique spectral features. These results allow us to define characteristic features that distinguish several different regimes of coupling in circuit-QED systems.
Superconducting flux qubits are a promising candidate for realizing quantum information processing and quantum simulations. Such devices behave like artificial atoms, with the advantagethat one can easily tune the „atoms“ internal properties. Here, by harnessing this flexibility, we propose a technique to minimize the inhomogeneous broadening of a large ensemble of flux qubits by tuning only the external flux. In addition, as an example of many-body physics in such an ensemble, we show how to observe superradiance, and its quadratic scaling with ensemble size, using a tailored microwave control pulse that takes advantage of the inhomogeneous broadening itself to excite only a sub-ensemble of the qubits. Our scheme opens up an approach to using superconducting circuits to explore the properties of quantum many-body systems.
The hybridization of distinct quantum systems is now seen as an effective way to engineer the properties of an entire system leading to applications in quantum metamaterials, quantumsimulation, and quantum metrology. One well known example is superconducting circuits coupled to ensembles of microscopic natural atoms. In such cases, the properties of the individual atom are intrinsic, and so are unchangeable. However, current technology allows us to fabricate large ensembles of macroscopic artificial atoms such as superconducting flux qubits, where we can really tailor and control the properties of individual qubits. Here, we demonstrate coherent coupling between a microwave resonator and several thousand superconducting flux qubits, where we observe a large dispersive frequency shift in the spectrum of 250 MHz induced by collective behavior. These results represent the largest number of coupled superconducting qubits realized so far. Our approach shows that it is now possible to engineer the properties of the ensemble, opening up the way for the controlled exploration of the quantum many-body system.
To control light-matter interaction at the single-quantum level in cavity quantum electrodynamics (cavity-QED) or circuit-QED, strong coupling between the light and matter componentsis indispensable. Specifically, the coupling rate g must be larger than the decay rates. If g is increased further and becomes as large as the frequencies of light and matter excitations, the energy eigenstates including the ground state are predicted to be highly entangled. This qualitatively new coupling regime can be called the deep strong-coupling regime. One approach toward the deep strong-coupling regime is to use huge numbers of identical systems to take advantage of ensemble enhancement. With the emergence of so-called macroscopic artificial atoms, superconducting qubits for example, it has become possible for a single artificial atom to realize ultrastrong coupling, where ℏg exceeds ~10% of the energies of the qubit ℏωq and the harmonic oscillator ℏωo. By making use of the macroscopic magnetic dipole moment of a flux qubit, large zero-point-fluctuation current of an LC oscillator, and large Josephson inductance of a coupler junction, we have realized circuits in the deep strong-coupling regime, where g/ωo ranges from 0.72 to 1.34 and g/ωq >> 1. Using energy spectroscopy measurements, we have observed unconventional transition spectra between Schrodinger cat-like energy eigenstates. These states involve quantum superpositions of Fock states with phase-space displacements of ±g/ωo and remarkably survive with environmental noise. Our results provide a basis for ground-state-based entangled-pair generation and open a new direction in circuit-QED.
One of the promising systems to realize quantum computation is a hybrid system where a superconducting flux qubit plays a role of a quantum processor and the NV center ensemble is usedas a quantum memory. We have theoretically and experimentally studied the effect of magnetic fields on this hybrid system, and found that the lifetime of the vacuum Rabi oscillation is improved by applying a few mT magnetic field to the NV center ensemble. Here, we construct a theoretical model to reproduce the vacuum Rabi oscillations with/without magnetic fields applied to the NV centers, and we determine the reason why magnetic fields can affect the coherent properties of the NV center ensemble. From our theoretical analysis, we quantitatively show that the magnetic fields actually suppress the inhomogeneous broadening from the strain in the NV centers.
Here, we propose a scheme to generate a controllable Ising interaction between superconducting flux qubits. Existing schemes rely on inducting couplings to realize Ising interactionsbetween flux qubits, and the interaction strength is controlled by an applied magnetic field On the other hand, we have found a way to generate an interaction between the flux qubits via capacitive couplings. This has an advantage in individual addressability, because we can control the interaction strength by changing an applied voltage that can be easily localized. This is a crucial step toward the realizing superconducting flux qubit quantum computation.
We have built a hybrid system composed of a superconducting flux qubit (the processor) and an ensemble of nitrogen-vacancy centers in diamond (the memory) that can be directly coupledto one another and demonstrated how information can be transferred from the flux qubit to the memory, stored and subsequently retrieved. We have established the coherence properties of the memory, and succeeded in creating an entangled state between the processor and memory, demonstrating how the entangled state’s coherence is preserved. Our results are a significant step towards using an electron spin ensemble as a quantum memory for superconducting qubits.